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    Metal-organic framework based mixed matrix membranes: a solution for highly efficient CO2 capture?

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    c4cs00437j.pdf (3.919Mb)
    Identifiers
    URI: http://hdl.handle.net/11556/180
    ISSN: 1460-4744
    DOI: 10.1039/c4cs00437j
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    Author/s
    Seoane, Beatriz; Coronas, Joaquin; Gascon, Ignacio; Etxeberria-Benavides, Miren; Karvan, Oguz; [et al.]
    Date
    2015
    Keywords
    hollow-fiber membranes
    hansen solubility parameters
    gas separation performance
    carbn-dioxide capture
    zeolitic imidazolate frameworks
    nano-composite membranes
    IGCC power-plants
    of-the-art
    nanocomposite membranes
    hydrogen separation
    Abstract
    The field of metal-organic framework based mixed matrix membranes (M(4)s) is critically reviewed, with special emphasis on their application in CO2 capture during energy generation. After introducing the most relevant parameters affecting membrane performance, we define targets in terms of selectivity and productivity based on existing literature on process design for pre- and post-combustion CO2 capture. Subsequently, the state of the art in M(4)s is reviewed against these targets. Because final application of these membranes will only be possible if thin separation layers can be produced, the latest advances in the manufacture of M-4 hollow fibers are discussed. Finally, the recent efforts in understanding the separation performance of these complex composite materials and future research directions are outlined.
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    article

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